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Mukai, Masayuki; Tanaka, Tadao; Maeda, Toshikatsu; Ogawa, Hiromichi; Matsumoto, Junko; Munakata, Masahiro; Zhao, Y.*; Guo, Z.*; Ni, S.*; Li, S.*
Nihon Genshiryoku Gakkai Wabun Rombunshi, 2(3), p.342 - 349, 2003/09
Evaluation of radionuclide migration in geologic media is of great importance in safety assessment for shallow land disposal specially for TRU nuclides because of inadequate data based on field test. As a cooperative research between JAERI and CIRP, a field test of radionuclide migration was conducted under natural condition using Sr-90, Np-237 and Pu-238 to obtain migration data of the radionuclides in actual aerated layer under natural rainfall condition. Values of input parameters to an existing evaluation equation of nuclide migration were determined on the basis of the results of laboratory experiments of batch and column methods and field investigation. Migration distribution of the radionuclides calculated with the determined values showed reasonable agreement with the measured distribution of the field test. This confirmed an applicability of the evaluation equation for radionuclide migration to actual aerated layer under natural condition.
Tanaka, Tadao; Mukai, Masayuki; Maeda, Toshikatsu; Matsumoto, Junko; Ogawa, Hiromichi; Li, S.*; Wang, Z.*; Wang, J.*; Guo, Z.*; Zhao, Y.*
JAERI-Research 2002-034, 20 Pages, 2002/12
Adsorption mechanisms and models of Sr(II), Np(V), Pu(IV) and Am(III) on the loess were investigated from their adsorption and desorption properties. The distribution coefficient of Sr and Np was 2 - 3 orders of magnitude smaller than that of Pu and Am. The adsorption of Sr and Np was mainly controlled by the ion exchange reaction. On the other hand, the adsorption of Pu and Am was mostly controlled by the selective chemical reactions with Fe and Mn oxyhydroxide/oxide and humic substances. On the basis of the experimental results, several types of adsorption models of the radionuclides, considering elemental concentrations, adsorption mechanisms and kinetics, were proposed for setting up the analytical systems of radionuclide migration in the loess media.
Umezawa, Hirokazu; ;
Journal of Nuclear Science and Technology, 13(6), p.327 - 332, 1976/06
Times Cited Count:17no abstracts in English